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Micropatterned Amorphous Zr-Based Alloys Coated with Silica Nanoparticles as Superhydrophobic Surfaces against Abrasion
Li, Mingjie1; Luo, Wenxin1; Sun, Haoyang1; Xu, Jingfu1; Ng, Kar Wei2; Cheng, Xing1
2021-11-26
Source PublicationACS Applied Nano Materials
ISSN2574-0970
Volume4Issue:11Pages:12300-12307
Abstract

Superhydrophobic metallic surfaces with mechanical stability as well as self-cleaning and anticorrosion functions are highly desirable because of their promising applications in various aspects. Large apparent water contact angles (≥150°) on metal surfaces are usually realized by high surface roughness and low surface energy. However, rough nanoscale features and low-energy coatings are prone to wear, causing degradation of the local wetting property during service. Herein, we develop a low-cost and scalable fabrication methodology to prepare composite superhydrophobic surfaces (water contact angle ∼154.7± 2.3° and sliding angle ∼1.2 ± 0.2°) by integrating a micropatterned amorphous alloy frame with functionalized nanoparticles. Amorphous interconnected microwalls provide augmented resistance against abrasion, whereas spray-coated nanomaterials residing within the frame impart water repellency. Metallic surfaces can withstand abrasion against sandpaper for 40 m under a local pressure of 120 kPa, before losing their perfect superhydrophobic performances. The composite surfaces also maintain its water repellency after mechanical bending, knife scratching, water impact jetting, ultraviolet (UV) irradiation, and acid immersion. We envisage that the design strategies here provide a practical route to manufacture water-repellent surfaces with metallic glass in harsh nautical applications.

KeywordImprint Micropatterns Amorphous Alloy Silica Nanoparticles Superhydrophobic Mechanical Stability Anti-abrasion
DOI10.1021/acsanm.1c02780
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaScience & Technology - Other Topics ; Materials Science
WOS SubjectNanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS IDWOS:000752894100092
PublisherAMER CHEMICAL SOC1155 16TH ST, NW, WASHINGTON, DC 20036
The Source to ArticlePB_Publication
Scopus ID2-s2.0-85119133928
Fulltext Access
Citation statistics
Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorLi, Mingjie; Cheng, Xing
Affiliation1.Department of Materials Science and Engineering, Southern University of Science and Technology, Shenzhen, 518055, China
2.Institute of Applied Physics and Materials Engineering, University of Macau, Taipa, 999078, Macao
Recommended Citation
GB/T 7714
Li, Mingjie,Luo, Wenxin,Sun, Haoyang,et al. Micropatterned Amorphous Zr-Based Alloys Coated with Silica Nanoparticles as Superhydrophobic Surfaces against Abrasion[J]. ACS Applied Nano Materials, 2021, 4(11), 12300-12307.
APA Li, Mingjie., Luo, Wenxin., Sun, Haoyang., Xu, Jingfu., Ng, Kar Wei., & Cheng, Xing (2021). Micropatterned Amorphous Zr-Based Alloys Coated with Silica Nanoparticles as Superhydrophobic Surfaces against Abrasion. ACS Applied Nano Materials, 4(11), 12300-12307.
MLA Li, Mingjie,et al."Micropatterned Amorphous Zr-Based Alloys Coated with Silica Nanoparticles as Superhydrophobic Surfaces against Abrasion".ACS Applied Nano Materials 4.11(2021):12300-12307.
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