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Close-loop recycling of perovskite solar cells through dissolution-recrystallization of perovskite by butylamine
Xiyuan Feng1,2; Qing Guo3; Jingwei Xiu1; Zhiqin Ying1,2; Kar Wei Ng2,4; Limin Huang3; Shuangpeng Wang2,4; Hui Pan2,4; Zikang Tang2,4; Zhubing He1
2021-02-24
Source PublicationCell Reports Physical Science
ISSN2666-3864
Volume2Issue:2Pages:100341
Abstract

Organic-inorganic lead halide perovskite solar cells (PSCs) have achieved impressive progress in both conversion efficiency and stability. However, the leakage risk of toxic lead in the fabrication and service of PSCs hinders their commercialization; hence, themanagement of lead is imperative. Here, we report a close-loop recycling strategy to collect the key materials involved in devices with butylamine (BA), even regenerating solar cells with recycled materials including perovskite absorbers and NiOx-coated ITO glass substrates. The regenerated devices show performance equivalent to that of fresh ones and nearly 18% PCE for the champions. The total recycling yield of lead is more than 98.9%. The recycling can be attributed to the unique interaction between lead halides and BA. Our strategy could move PSCs toward commercialization by effective close-loop recycling and refabrication of whole PSC devices.

KeywordPerovskite Solar Cells Lead Lead Recycling Dissolution Recrystallization Recycling Amines Coordination Liquefaction
DOI10.1016/j.xcrp.2021.100341
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaChemistry ; Energy & Fuels ; Materials Science ; Physics
WOS SubjectChemistry, Multidisciplinary ; Energy & Fuels ; Materials Science, Multidisciplinary ; Physics, Multidisciplinary
WOS IDWOS:000658762100021
The Source to ArticlePB_Publication
Scopus ID2-s2.0-85101160179
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Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorShuangpeng Wang; Zhubing He
Affiliation1.Department of Materials Science and Engineering,Shenzhen Key Laboratory of Full Spectral Solar Electricity Generation (FSSEG),Southern University of Science and Technology,Shenzhen,No. 1088, Xueyuan Rd.,518055,China
2.Joint Key Laboratory of the Ministry of Education,Institute of Applied Physics and Materials Engineering,University of Macau,Avenida da Universidade,Taipa,999078,China
3.Department of Chemistry,Southern University of Science and Technology,Shenzhen,No. 1088, Xueyuan Rd.,518055,China
4.Department of Physics and Chemistry,Faculty of Science and Technology,University of Macau,Avenida da Universidade,Taipa,999078,China
First Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING;  Faculty of Science and Technology
Recommended Citation
GB/T 7714
Xiyuan Feng,Qing Guo,Jingwei Xiu,et al. Close-loop recycling of perovskite solar cells through dissolution-recrystallization of perovskite by butylamine[J]. Cell Reports Physical Science, 2021, 2(2), 100341.
APA Xiyuan Feng., Qing Guo., Jingwei Xiu., Zhiqin Ying., Kar Wei Ng., Limin Huang., Shuangpeng Wang., Hui Pan., Zikang Tang., & Zhubing He (2021). Close-loop recycling of perovskite solar cells through dissolution-recrystallization of perovskite by butylamine. Cell Reports Physical Science, 2(2), 100341.
MLA Xiyuan Feng,et al."Close-loop recycling of perovskite solar cells through dissolution-recrystallization of perovskite by butylamine".Cell Reports Physical Science 2.2(2021):100341.
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