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Quantum dots enhanced stability of in-situ fabricated perovskite nanocrystals based light-emitting diodes: Electrical field distribution effects
Xue, Xulan1; Li, Menglin2; Liu, Zhenjie1; Wang, Chenhui2; Xu, Jincheng3; Wang, Shuangpeng3; Zhang, Hanzhuang1; Zhong, Haizheng2; Ji, Wenyu1
2022
Source PublicationFundamental Research
ISSN2096-9457
Abstract

With the development in fabricating efficient perovskite light emitting diodes (PeLEDs), improving the operating stability becomes an urgent task. Here we report quantum dot (QD) enhanced stability of PeLEDs by introducing CdSe/ZnS core-shell QDs in toluene anti-solvent during in-situ fabrication of FAPbBr perovskite nanocrystals (PNCs) films. In comparison with PNC films with pristine toluene as the anti-solvent, the as-prepared FAPbBr PNC films with a QD monolayer on the surface exhibit improved photoluminescence quantum yield, enhanced photostability and better reproducibility. Benefiting from these advantages, the peak luminance and the maximum external quantum efficiency of the PeLED containing QD monolayer are increased from 6807 cd/m to 86670 cd/m and 2.4% to 7.1%, respectively. The T lifetime under the initial luminance of 1021 cd/m approaches 83 minutes. Based on electrical field simulation and transient electroluminescence measurements, the enhanced stability can be mainly attributed to the electrical field redistribution induced by the QD monolayer. This work demonstrates that the combination of QDs and perovskites provides an effective strategy to address the operational stability of PeLEDs. The insights into electrical field distribution effect will make great impact on stability improvement of other perovskite based devices.

KeywordElectrical Field Distribution Light-emitting Diodes Operational Stability Perovskite Nanocrystals Quantum Dots
DOI10.1016/j.fmre.2022.08.004
URLView the original
Language英語English
Scopus ID2-s2.0-85143868738
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Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Co-First AuthorXue, Xulan
Corresponding AuthorZhong, Haizheng; Ji, Wenyu
Affiliation1.Key Lab of Physics and Technology for Advanced Batteries (Ministry of Education), College of Physics, Jilin University, Changchun, 130012, China
2.MIIT Key Laboratory for Low-Dimensional Quantum Structure and Devices, School of Materials Science & Engineering, Beijing Institute of Technology, Beijing, 100081, China
3.Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, Macau SAR, 999078, China
Recommended Citation
GB/T 7714
Xue, Xulan,Li, Menglin,Liu, Zhenjie,et al. Quantum dots enhanced stability of in-situ fabricated perovskite nanocrystals based light-emitting diodes: Electrical field distribution effects[J]. Fundamental Research, 2022.
APA Xue, Xulan., Li, Menglin., Liu, Zhenjie., Wang, Chenhui., Xu, Jincheng., Wang, Shuangpeng., Zhang, Hanzhuang., Zhong, Haizheng., & Ji, Wenyu (2022). Quantum dots enhanced stability of in-situ fabricated perovskite nanocrystals based light-emitting diodes: Electrical field distribution effects. Fundamental Research.
MLA Xue, Xulan,et al."Quantum dots enhanced stability of in-situ fabricated perovskite nanocrystals based light-emitting diodes: Electrical field distribution effects".Fundamental Research (2022).
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