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Type-II antiferromagnetic ordering in the double perovskite oxide Sr2NiWO6
LI HAIFENG2; Cheng Su1; Xu-Tao Zeng1; Kaitong Sun2; Denis Sheptyakov3; Ziyu Chen1; Xian-Lei Sheng1; Wentao Jin1
2023-08-10
Source PublicationPhysical Review B
ISSN2469-9969
Volume108Issue:5Pages:054416
Abstract

Magnetic double perovskite (DP) compounds provide a fertile playground to explore interesting electronic and magnetic properties. By complementary macroscopic characterizations, neutron powder diffraction measurements, and first-principles calculations, we have performed comprehensive studies on the magnetic ordering in the DP compound Sr2NiWO6. It is found by neutron diffraction to order magnetically in a collinear type-II antiferromagnetic (AFM) structure in a tetragonal lattice with k=(0.5,0,0.5) below TN=56K. In the ground state, the ordered moment of the spin-1 Ni2+ ions is determined to be 1.9(2)µB, indicating a significant quenching of the orbital moment. The Ni2+ moments in Sr2NiWO6 are revealed to cant off the c axis by 29.2∘, which is well supported by the first-principles magnetic anisotropy energy calculations. Furthermore, the in-plane and out-of-plane next-nearest-neighbor superexchange couplings (J2 and J2c) are found to play a dominant role in the spin Hamiltonian of Sr2NiWO6, which accounts for the stabilization of the type-II AFM structure as its magnetic ground state.

DOI10.1103/PhysRevB.108.054416
URLView the original
Indexed BySCIE
Language英語English
PublisherAmerican Physical Society
Scopus ID2-s2.0-85167946042
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Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorLI HAIFENG; Wentao Jin
Affiliation1.School of Physics, Beihang University, Beijing 100191, China
2.Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, Macao SAR 999078, China
3.Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institut, CH-5232 Villigen-PSI, Switzerland
First Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
LI HAIFENG,Cheng Su,Xu-Tao Zeng,et al. Type-II antiferromagnetic ordering in the double perovskite oxide Sr2NiWO6[J]. Physical Review B, 2023, 108(5), 054416.
APA LI HAIFENG., Cheng Su., Xu-Tao Zeng., Kaitong Sun., Denis Sheptyakov., Ziyu Chen., Xian-Lei Sheng., & Wentao Jin (2023). Type-II antiferromagnetic ordering in the double perovskite oxide Sr2NiWO6. Physical Review B, 108(5), 054416.
MLA LI HAIFENG,et al."Type-II antiferromagnetic ordering in the double perovskite oxide Sr2NiWO6".Physical Review B 108.5(2023):054416.
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