Residential College | false |
Status | 已發表Published |
Promoted Electronic Coupling of Acoustic Phonon Modes in Doped Semimetallic MoTe2 | |
Cui, Xiangyue1; Yan, Hejin1; Yan, Xuefei4,5; Zhou, Kun2,3; Cai, Yongqing1 | |
2023-09-12 | |
Source Publication | ACS Nano |
ISSN | 1936-0851 |
Volume | 17Issue:17Pages:16530-16538 |
Abstract | As a prototype of the Weyl superconductor, layered molybdenum ditelluride (MoTe) encompasses two semimetallic phases (1T′ and T) which differentiate from each other via a slight tilting of the out-of-plane lattice. Both phases are subjected to serious phase mixing, which complicates the analysis of its origin of superconductivity. Herein, we explore the electron-phonon coupling (EPC) of the monolayer semimetallic MoTe, without phase ambiguity under this thickness limit. Apart from the hardening or softening of the phonon modes, the strength of the EPC can be strongly modulated by doping. Specifically, longitudinal and out-of-plane acoustic modes are significantly activated for electron doped MoTe. This is ascribed to the presence of rich valley states and equispaced nesting bands, which are dynamically populated under charge doping. Through comparing the monolayer and bilayer MoTe, the strength of EPC is found to be less likely to depend on thickness for neutral samples but clearly promoted for thinner samples with electron doping, while for hole doping, the strength alters more significantly with the thickness than doping. Our work explains the issue of the doping sensitivity of the superconductivity in semimetallic MoTe and establishes the critical role of activating acoustic phonons in such low-dimensional materials. |
Keyword | Charge Doping Electron−phonon Coupling First-principles Calculation Molybdenum Ditelluride Superconductivity Two-dimensional Materials |
DOI | 10.1021/acsnano.3c01229 |
URL | View the original |
Indexed By | SCIE |
Language | 英語English |
WOS Research Area | Chemistry ; Science & Technology - Other Topics ; Materials Science |
WOS Subject | Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
WOS ID | WOS:001122019300001 |
Publisher | AMER CHEMICAL SOC, 1155 16TH ST, NW, WASHINGTON, DC 20036 |
Scopus ID | 2-s2.0-85171202686 |
Fulltext Access | |
Citation statistics | |
Document Type | Journal article |
Collection | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING |
Corresponding Author | Cai, Yongqing |
Affiliation | 1.Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Taipa, 999078, Macao 2.School of Mechanical and Aerospace Engineering, Nanyang Technological University, 50 Nanyang Avenue, 639798, Singapore 3.Environmental Process Modelling Centre, Nanyang Environment and Water Research Institute, Nanyang Technological University, 1 Cleantech Loop, 637141, Singapore 4.School of Microelectronics Science and Technology, Sun Yat-Sen University, Zhuhai, 519082, China 5.Guangdong Provincial Key Laboratory of Optoelectronic Information Processing Chips and Systems, Sun Yat-Sen University, Zhuhai, 519082, China |
First Author Affilication | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING |
Corresponding Author Affilication | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING |
Recommended Citation GB/T 7714 | Cui, Xiangyue,Yan, Hejin,Yan, Xuefei,et al. Promoted Electronic Coupling of Acoustic Phonon Modes in Doped Semimetallic MoTe2[J]. ACS Nano, 2023, 17(17), 16530-16538. |
APA | Cui, Xiangyue., Yan, Hejin., Yan, Xuefei., Zhou, Kun., & Cai, Yongqing (2023). Promoted Electronic Coupling of Acoustic Phonon Modes in Doped Semimetallic MoTe2. ACS Nano, 17(17), 16530-16538. |
MLA | Cui, Xiangyue,et al."Promoted Electronic Coupling of Acoustic Phonon Modes in Doped Semimetallic MoTe2".ACS Nano 17.17(2023):16530-16538. |
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