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Interface Engineering on Constructing Physical and Chemical Stable Solid-State Electrolyte Toward Practical Lithium Batteries
He, Honggang1; Wang, Litong2; Al-Abbasi, Malek1; Cao, Chunyan1,3; Li, Heng4; Xu, Zhu4; Chen, Shi4; Zhang, Wei1; Li, Ruiqing1; Lai, Yuekun5; Tang, Yuxin5; Ge, Mingzheng1,4
2024-07-01
Source PublicationEnergy and Environmental Materials
ISSN2575-0348
Volume7Issue:4
AbstractSolid-state lithium batteries (SSLBs) with high safety have emerged to meet the increasing energy density demands of electric vehicles, hybrid electric vehicles, and portable electronic devices. However, the dendrite formation, high interfacial resistance, and deleterious interfacial reactions caused by solid–solid contact between electrode and electrolyte have hindered the commercialization of SSLBs. Thus, in this review, the state-of-the-art developments in the rational design of solid-state electrolyte and their progression toward practical applications are reviewed. First, the origin of interface instability and the sluggish charge carrier transportation in solid–solid interface are presented. Second, various strategies toward stabilizing interfacial stability (reducing interfacial resistance, suppressing lithium dendrites, and side reactions) are summarized from the physical and chemical perspective, including building protective layer, constructing 3D and gradient structures, etc. Finally, the remaining challenges and future development trends of solid-state electrolyte are prospected. This review provides a deep insight into solving the interfacial instability issues and promising solutions to enable practical high-energy-density lithium metal batteries.
Keyworddendrite formation high energy density interface instability interfacial resistance solid-state electrolyte
DOI10.1002/eem2.12699
URLView the original
Language英語English
Scopus ID2-s2.0-85182665230
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Document TypeJournal article
CollectionUniversity of Macau
Affiliation1.School of Textile and Clothing, Nantong University, Nantong, Jiangsu, 226019, China
2.School of Science, Qingdao University of Technology, Qingdao, Shandong, 266520, China
3.Department of Biomedical Sciences, City University of Hong Kong, 999077, Hong Kong
4.Institute of Applied Physics and Materials Engineering, University of Macau, 999078, Macao
5.College of Chemical Engineering, Fuzhou University, Fuzhou, Fujian, 350116, China
Recommended Citation
GB/T 7714
He, Honggang,Wang, Litong,Al-Abbasi, Malek,et al. Interface Engineering on Constructing Physical and Chemical Stable Solid-State Electrolyte Toward Practical Lithium Batteries[J]. Energy and Environmental Materials, 2024, 7(4).
APA He, Honggang., Wang, Litong., Al-Abbasi, Malek., Cao, Chunyan., Li, Heng., Xu, Zhu., Chen, Shi., Zhang, Wei., Li, Ruiqing., Lai, Yuekun., Tang, Yuxin., & Ge, Mingzheng (2024). Interface Engineering on Constructing Physical and Chemical Stable Solid-State Electrolyte Toward Practical Lithium Batteries. Energy and Environmental Materials, 7(4).
MLA He, Honggang,et al."Interface Engineering on Constructing Physical and Chemical Stable Solid-State Electrolyte Toward Practical Lithium Batteries".Energy and Environmental Materials 7.4(2024).
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