Residential College | false |
Status | 已發表Published |
Visible-Light-Excited Fluorescent Hydrogel Tapes for Dual-Channel Copper Ions Recognition | |
Yuan, Zihao1; Zhu, Canjie2; Huang, Guang3; Lei, Bing1; Wu, Mingmei1; Feng, Zhiyuan1; Yang, Zhiyong4; Wei, Qiang5; Meng, Guozhe1; Guo, Honglei1 | |
2024-09 | |
Source Publication | ACS Applied Polymer Materials |
ISSN | 2637-6105 |
Volume | 6Issue:17Pages:10467-10477 |
Abstract | Incorporating aggregation-induced emission (AIE) molecules into hydrogels that exhibit ion-responsive and visible light excitation while maintaining good luminescence is challenging. To address this, we designed an ion-sensitive fluorescent hydrogel using an aggregation-induced phase separation strategy. We synthesized a tetraphenylethylene derivative (TPEBPy) with a long-chain alkene and copolymerized it with hydroxyethyl methacrylate (HEMA) and acrylic acid (AAc) through free-radical copolymerization. Because of the extended π-conjugated structure and AIE effect of the TPEBPy molecules, the synthesized fluorescent p(HEMA-co-AAc-TPEBPy) hydrogels exhibit excitation in the visible range (415 nm).This strategy requires only 0.1 mol % of TPEBPy molecules to achieve a sensitive threshold for specific recognition of copper ions as low as 10-5 M. By analyzing the fluorescence lifetime results, we determined the distribution of fluorescent molecules within the hydrogel, distinguishing between the aggregated and dispersed states. Additionally, this fluorescent hydrogel demonstrates the capability for visual colorimetric and fluorescence dual-channel detection of copper ions. |
Keyword | Aggregation-induced Emission Early Warning Of Corrosion Fluorescent Hydrogel Reusability Visible Light Excitation |
DOI | 10.1021/acsapm.4c01622 |
URL | View the original |
Indexed By | SCIE |
Language | 英語English |
WOS Research Area | Materials Science ; Polymer Science |
WOS Subject | Materials Science, Multidisciplinary ; Polymer Science |
WOS ID | WOS:001308499200001 |
Publisher | AMER CHEMICAL SOC, 1155 16TH ST, NW, WASHINGTON, DC 20036 |
Scopus ID | 2-s2.0-85202730352 |
Fulltext Access | |
Citation statistics | |
Document Type | Journal article |
Collection | Faculty of Science and Technology |
Corresponding Author | Feng, Zhiyuan; Yang, Zhiyong; Wei, Qiang; Meng, Guozhe; Guo, Honglei |
Affiliation | 1.School of Chemical Engineering and Technology, Sun Yat-sen Universit, Zhuhai, 519082, China 2.School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou, 510006, China 3.Faculty of Science and Technology, University of Macau, 999078, Macao 4.Key Laboratory for Polymeric Composite and Functional Materials, Ministry of Education, School of Chemistry, Sun Yat-sen University, Guangzhou, 510275, China 5.Ningbo Institute of Materials Technology and Engineering (NIMTE), Chinese Academy of Sciences (CAS), Ningbo, 315201, China |
Recommended Citation GB/T 7714 | Yuan, Zihao,Zhu, Canjie,Huang, Guang,et al. Visible-Light-Excited Fluorescent Hydrogel Tapes for Dual-Channel Copper Ions Recognition[J]. ACS Applied Polymer Materials, 2024, 6(17), 10467-10477. |
APA | Yuan, Zihao., Zhu, Canjie., Huang, Guang., Lei, Bing., Wu, Mingmei., Feng, Zhiyuan., Yang, Zhiyong., Wei, Qiang., Meng, Guozhe., & Guo, Honglei (2024). Visible-Light-Excited Fluorescent Hydrogel Tapes for Dual-Channel Copper Ions Recognition. ACS Applied Polymer Materials, 6(17), 10467-10477. |
MLA | Yuan, Zihao,et al."Visible-Light-Excited Fluorescent Hydrogel Tapes for Dual-Channel Copper Ions Recognition".ACS Applied Polymer Materials 6.17(2024):10467-10477. |
Files in This Item: | There are no files associated with this item. |
Items in the repository are protected by copyright, with all rights reserved, unless otherwise indicated.
Edit Comment