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Ultrahigh “relative energy density” and mass loading of carbon cloth anodes for K-ion batteries
Xie, Junpeng1,2; Li, Jinliang1; Li, Xiaodan1; Lei, Hang1,3; Zhuo, Wenchen1,3; Li, Xibo1; Hong, Guo2; Hui, Kwun Nam2; Pan, Likun4; Mai, Wenjie1
2021-02-01
Source PublicationCCS Chemistry
ISSN2096-5745
Volume3Issue:2Pages:791-799
Abstract

Mass loading and potential plateau are the two most important issues of potassium (K)-ion batteries (KIBs), but they have long been ignored in previous studies. Herein, we report a simple and scalable method to fabricate acidized carbon clothes (A-CC) as high mass loading (13.1 mg cm) anode for KIBs, which achieved a reversible areal-specific capacity of 1.81 mAh cm at 0.2 mA cm. Besides, we have proposed the concept of “relative energy density” to reasonably evaluate the electrochemical performance of the anode. According to our calculation method, the A-CC electrode exhibited an ultrahigh relative energy density of 46 Wh m in the initial charge process and remained at 40 Wh m after 50 cycles. Furthermore, we performed the operando Raman spectroscopy (ORS) to investigate the K-ion storage mechanism. We believe that our work might provide a new guideline for the evaluation of anode performance, thereby, opening an avenue for the development of commercial anode.

KeywordAcidized Carbon Clothes High Mass Loading K-ion Batteries Operando Raman Spectra Relative Energy Density
DOI10.31635/ccschem.020.202000203
URLView the original
Indexed ByESCI
Language英語English
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
WOS IDWOS:000794136000009
PublisherCHINESE CHEMICAL SOCC/O DEPT INT AFFAIRS, SECRETARY OF CHEM SOC, PO BOX 2709, BEIJING 100080, PEOPLES R CHINA
Scopus ID2-s2.0-85107647719
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Citation statistics
Document TypeJournal article
CollectionFaculty of Science and Technology
INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
DEPARTMENT OF PHYSICS AND CHEMISTRY
Corresponding AuthorLi, Jinliang; Mai, Wenjie
Affiliation1.Siyuan Laboratory, Guangdong Provincial Engineering Technology Research Center of Vacuum Coating Technologies and New Materials, Department of Physics, Jinan University, Guangzhou, 510632, China
2.Institute of Applied Physics and Materials Engineering (IAPME), University of Macau, Department of Physics and Chemistry, Faculty of Science and Technology, University of Macau, Macao, 999078, Macao
3.Department of Chemistry, Jinan University, Guangzhou, 510632, China
4.Shanghai Key Laboratory of Magnetic Resonance, School of Physics and Electronic Science, East China Normal University, Shanghai, 200062, China
First Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
Xie, Junpeng,Li, Jinliang,Li, Xiaodan,et al. Ultrahigh “relative energy density” and mass loading of carbon cloth anodes for K-ion batteries[J]. CCS Chemistry, 2021, 3(2), 791-799.
APA Xie, Junpeng., Li, Jinliang., Li, Xiaodan., Lei, Hang., Zhuo, Wenchen., Li, Xibo., Hong, Guo., Hui, Kwun Nam., Pan, Likun., & Mai, Wenjie (2021). Ultrahigh “relative energy density” and mass loading of carbon cloth anodes for K-ion batteries. CCS Chemistry, 3(2), 791-799.
MLA Xie, Junpeng,et al."Ultrahigh “relative energy density” and mass loading of carbon cloth anodes for K-ion batteries".CCS Chemistry 3.2(2021):791-799.
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