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High performance broadband photo and soft X-ray detectors based on two dimensional CrSiTe3
Li, Yun1; Liu, Jingying1; Su, Xin2; Ou, Qingdong1; Wan, Zhichen1; Wu, Yingjie1; Yu, Wenzhi1; Bao, Xiaozhi3; Huang, Yamin4; Wang, Xiaomu2; Tadich, Anton5; Shabbir, Babar1,6; Bao, Qiaoliang1
2020-05-28
Source PublicationJournal of Materials Chemistry C
ISSN2050-7526
Volume8Issue:20Pages:6659-6666
Other Abstract

Broadband photodetectors are essential for various applications including spectroscopy, communication, imaging and sensing. Even though few materials show broadband photodetection, they are only capable of detecting light in limited spectral ranges from infrared (IR) to ultraviolet (UV) wavelengths. However, their functionalities at much shorter wavelengths such as ionizing radiation still present a challenge because of the limitations from the material properties. Here we demonstrate a room temperature, high performance broadband photodetector based on van der Waals (vdWs) magnetic material CrSiTe(CST) that can efficiently detect both soft X-rays and light in the near-infrared (NIR) and visible wavelength ranges. The CrSiTebased device can work with a high sensitivity (˜463 µC Gycm) under synchrotron soft X-rays, which is more than twenty times more sensitive than the conventional a-Se device. In the NIR range, the device can achieve a maximum responsivity of around 206 A Wat 785 nm, an extremely high external quantum efficiency (EQE) of 32600%, a detectivity of 1.25 × 10cm HzWand a relatively fast photoresponse time (rise time ~43 ms under X-rays, 17 ms under a 785 nm laser). Together these results demonstrate a high-performance broadband photo and X-ray detector, offering intriguing opportunities for novel optoelectronic applications.

DOI10.1039/d0tc01354d
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaMaterials Science ; Physics
WOS SubjectMaterials Science, Multidisciplinary ; Physics, Applied
WOS IDWOS:000538108200003
PublisherROYAL SOC CHEMISTRY, THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND
Scopus ID2-s2.0-85085593568
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Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorShabbir, Babar; Bao, Qiaoliang
Affiliation1.Department of Materials Science and Engineering, and ARC Centre of Excellence in Future Low-Energy Electronics Technologies (FLEET), Monash University, Clayton, 3800, Australia
2.School of Electronic Science and Engineering, Nanjing University, Nanjing, 210093, China
3.Institute of Applied Physics and Materials Engineering (IAPME), University of Macau, Taipa, Macao
4.State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai, 865 Changning Road, 200050, China
5.Australian Synchrotron, ANSTO, Clayton, 800 Blackburn Road, 3168, Australia
6.Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province, College of Electronic Science and Technology and College of Optoelectronics Engineering, Shenzhen University, Shenzhen, 518060, China
Recommended Citation
GB/T 7714
Li, Yun,Liu, Jingying,Su, Xin,et al. High performance broadband photo and soft X-ray detectors based on two dimensional CrSiTe3[J]. Journal of Materials Chemistry C, 2020, 8(20), 6659-6666.
APA Li, Yun., Liu, Jingying., Su, Xin., Ou, Qingdong., Wan, Zhichen., Wu, Yingjie., Yu, Wenzhi., Bao, Xiaozhi., Huang, Yamin., Wang, Xiaomu., Tadich, Anton., Shabbir, Babar., & Bao, Qiaoliang (2020). High performance broadband photo and soft X-ray detectors based on two dimensional CrSiTe3. Journal of Materials Chemistry C, 8(20), 6659-6666.
MLA Li, Yun,et al."High performance broadband photo and soft X-ray detectors based on two dimensional CrSiTe3".Journal of Materials Chemistry C 8.20(2020):6659-6666.
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