| Residential College | false |
| Status | 已發表Published |
| Boosting the polysulfides adsorption-catalysis process on carbon nanotube interlayer via a simple polyelectrolyte-assisted strategy for high-performance lithium sulfur batteries | |
Fan, Xuliang1 ; Wang, Yongyin1; Zeng, Meng1; He, Huimin1; Huang, Jianyi1; Feng, Ziwen1; Li, Jing2; Liang, Zhongxin3; Zhou, Tao1
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| 2022-02-15 | |
| Source Publication | Journal of Alloys and Compounds
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| ISSN | 0925-8388 |
| Volume | 894Pages:162556 |
| Abstract | The introduction of conductive interlayer is an effective strategy to improve the sulfur utilization and restrict the migration of polysulfides for high-performance Li-S battery. Herein, a multifunctional CNT based interlayer was obtained by a simple polyelectrolyte (PDDA-TFSI) modified method. Due to the electro-positivity of PDDA-TFSI and the electronic coupling between CNT and PDDA-TFSI, the CNT/PDDA-TFSI interlayer exhibits a strong adsorption and effective catalysis towards polysulfides. Furthermore, the continuous CNT network ensures the successful electron transport during the charge-discharge process. As expected, the electrochemical properties of Li-S battery can be promoted significantly with the assistance of CNT/PDDA-TFSI interlayer. Even after 300 cycles, the CNT/PDDA-TFSI interlayer-based Li-S battery also delivers a higher capacity retention of 79.2%, proceeding Li-S batteries with and without CNT interlayer. This work proves that CNT/PDDA-TFSI film as a multifunctional interlayer has a promising application in advanced Li-S battery. |
| Keyword | Carbon Nanotube Lithium Sulfur Battery Multifunctional Interlayer Polyelectrolyte |
| DOI | 10.1016/j.jallcom.2021.162556 |
| URL | View the original |
| Indexed By | SCIE |
| Language | 英語English |
| WOS Research Area | Chemistry ; Materials Science ; Metallurgy & Metallurgical Engineering |
| WOS Subject | Chemistry, Physical ; Materials Science, Multidisciplinary ; Metallurgy & Metallurgical Engineering |
| WOS ID | WOS:000720139200002 |
| Publisher | ELSEVIER SCIENCE SAPO BOX 564, 1001 LAUSANNE, SWITZERLAND |
| Scopus ID | 2-s2.0-85118547595 |
| Fulltext Access | |
| Citation statistics | |
| Document Type | Journal article |
| Collection | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING |
| Corresponding Author | Fan, Xuliang; Li, Jing; Zhou, Tao |
| Affiliation | 1.School of Chemistry and Chemical Engineering, Key Laboratory of Clean Energy Materials Chemistry of Guangdong Higher Education Institutes, Research Center for Clean Energy Materials Chemical Engineering Technology of Guangdong, Institute of Physical Chemis 2.Guangdong-Hong Kong-Macau Joint Laboratory for Photonic-Thermal-Electrical Energy Materials and Devices, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, China 3.Department of Physics, University of Houston, Houston, 77204, United States |
| Corresponding Author Affilication | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING |
| Recommended Citation GB/T 7714 | Fan, Xuliang,Wang, Yongyin,Zeng, Meng,et al. Boosting the polysulfides adsorption-catalysis process on carbon nanotube interlayer via a simple polyelectrolyte-assisted strategy for high-performance lithium sulfur batteries[J]. Journal of Alloys and Compounds, 2022, 894, 162556. |
| APA | Fan, Xuliang., Wang, Yongyin., Zeng, Meng., He, Huimin., Huang, Jianyi., Feng, Ziwen., Li, Jing., Liang, Zhongxin., & Zhou, Tao (2022). Boosting the polysulfides adsorption-catalysis process on carbon nanotube interlayer via a simple polyelectrolyte-assisted strategy for high-performance lithium sulfur batteries. Journal of Alloys and Compounds, 894, 162556. |
| MLA | Fan, Xuliang,et al."Boosting the polysulfides adsorption-catalysis process on carbon nanotube interlayer via a simple polyelectrolyte-assisted strategy for high-performance lithium sulfur batteries".Journal of Alloys and Compounds 894(2022):162556. |
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