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Modulating thermal transport in a porous carbon honeycomb using cutting and deformation techniques
Han, Yang1; Zhao, Chaoxiang1; Bai, Hao1; Li, Yanjun1; Yang, Jiayue2; Chen, Yi Tung3; Hong, Guo4,5; Lacroix, David6; Isaiev, Mykola7
2022-02-07
Source PublicationPHYSICAL CHEMISTRY CHEMICAL PHYSICS
ISSN1463-9076
Volume24Issue:5Pages:3207-3215
Abstract

During the past few years, there has been a flurry of investigations on the lattice thermal transport of three-dimensional (3D) graphene, however, few studies have detailed how to adjust this property effectively using the presently available engineering technologies. In this work, the thermal transport properties of a porous single layer carbon honeycomb (SL-dCHC-2) and its mechanical response are systematically studied. We show that the thermal conductivity of SL-dCHC-2 can be adjusted effectively by varying the tensile strain, and its value is enhanced by up to 11.3 times with 8% strain as compared to the unstrained case. This value is significantly larger than what was observed for other two-dimensional (2D) materials such as silicene (∼7 times larger). This outstanding behavior is explained by the phonon mode level, indicating that a profound increase of the thermal conductivity under tensile strain is attributed to the enhancement of the phonon lifetime. In addition, the trend for the root mean squared displacement, which is closely related to the phonon anharmonic effect, correlates with the non-monotonic response of the dimerized C-C bonds at the linkage of the structure. These investigations and obtained results provide important guidance to develop 3D carbon honeycombs for several different purposes, such as for use as molecular sieves and in water purification applications.

DOI10.1039/d1cp04210f
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaChemistry ; Physics
WOS SubjectChemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS IDWOS:000744147600001
PublisherROYAL SOC CHEMISTRYTHOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND
Scopus ID2-s2.0-85124056842
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Citation statistics
Document TypeJournal article
CollectionFaculty of Science and Technology
INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
DEPARTMENT OF PHYSICS AND CHEMISTRY
Corresponding AuthorHan, Yang
Affiliation1.College of Power and Energy Engineering, Harbin Engineering University, Harbin, 150001, China
2.School of Energy and Power Engineering, Shandong University, Shandong, Jinan, 250061, China
3.Department of Mechanical Engineering, University of Nevada, Las Vegas, 89154, United States
4.Institute of Applied Physics and Materials Engineering, University of Macau, Taipa, Avenida da Universidade, 999078, Macao
5.Department of Physics and Chemistry, Faculty of Science and Engineering, University of Macau, Taipa, Avenida da Universidade, 999078, Macao
6.Université de Lorraine, CNRS, LEMTA, Nancy, F-54500, France
7.Faculty of Physics, Taras Shevchenko National University of Kyiv, Kyiv, 64/13, Volodymrska str., 01601, Ukraine
Recommended Citation
GB/T 7714
Han, Yang,Zhao, Chaoxiang,Bai, Hao,et al. Modulating thermal transport in a porous carbon honeycomb using cutting and deformation techniques[J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2022, 24(5), 3207-3215.
APA Han, Yang., Zhao, Chaoxiang., Bai, Hao., Li, Yanjun., Yang, Jiayue., Chen, Yi Tung., Hong, Guo., Lacroix, David., & Isaiev, Mykola (2022). Modulating thermal transport in a porous carbon honeycomb using cutting and deformation techniques. PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 24(5), 3207-3215.
MLA Han, Yang,et al."Modulating thermal transport in a porous carbon honeycomb using cutting and deformation techniques".PHYSICAL CHEMISTRY CHEMICAL PHYSICS 24.5(2022):3207-3215.
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