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Recent Advances in Electrocatalysts for Efficient Nitrate Reduction to Ammonia
Liu, Di1; Qiao, Lulu1; Peng, Shuyang2; Bai, Haoyun1; Liu, Chunfa1; Ip, Weng Fai3; Lo, Kin Ho2; Liu, Hongchao1; Ng, Kar Wei1,3; Wang, Shuangpeng1,3; Yang, Xiaozhan4; Pan, Hui1,3
2023-10-18
Source PublicationAdvanced Functional Materials
ISSN1616-301X
Volume33Issue:43
AbstractAmmonia as an irreplaceable chemical has been widely demanded to keep the sustainable development of the modern society. However, its industrial production consumes huge energy and releases extraordinary green-house gases, leading to various environmental issues. To achieve the green production of ammonia is a great challenge that has been extensively pursued recently. In the review, a most promising strategy, electrochemical nitrate reduction reaction (e-NORR) for the purpose is comprehensively investigated to give a full understanding of its development and mechanism and provide guidance for future directions. Particularly, the development of electrocatalysts is focused to realize the high ammonia yield rate and Faraday efficiency for industrial applications. The recent-developed catalysts, including noble metallic materials, alloys, metal compounds, single-metal-atom catalysts, and metal-free materials, are systematically discussed to review the effects of various factors on the catalytic performance in e-NORR. Accordingly, the strategies, including defects engineering, coordination environment modulating, surface controlling, and hybridization, are carefully discussed to improve the catalytic performance, such as the intrinsic activity and selectivity. Finally, perspectives and challenges are given out. This review shall provide insightful guidance on the development of advanced catalytic systems for the production of green ammonia efficiently in the industry.
KeywordElectrocatalysis Green Ammonia Production Nitrate Reduction
DOI10.1002/adfm.202303480
URLView the original
Indexed BySCIE
Language英語English
Scopus ID2-s2.0-85163183647
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Document TypeJournal article
CollectionDEPARTMENT OF PHYSICS AND CHEMISTRY
INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
DEPARTMENT OF ELECTROMECHANICAL ENGINEERING
Affiliation1.Institute of Applied Physics and Materials Engineering, University of Macau, Taipa, SAR, 999078, Macao
2.Department of Electromechanical Engineering, Faculty of Science and Technology, University of Macau, Taipa, SAR, 999078, Macao
3.Department of Physics and Chemistry, Faculty of Science and Technology, University of Macau, Taipa, SAR, 999078, Macao
4.Department of Physics and Energy, Chongqing University of Technology, Chongqing, 400054, China
First Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
Liu, Di,Qiao, Lulu,Peng, Shuyang,et al. Recent Advances in Electrocatalysts for Efficient Nitrate Reduction to Ammonia[J]. Advanced Functional Materials, 2023, 33(43).
APA Liu, Di., Qiao, Lulu., Peng, Shuyang., Bai, Haoyun., Liu, Chunfa., Ip, Weng Fai., Lo, Kin Ho., Liu, Hongchao., Ng, Kar Wei., Wang, Shuangpeng., Yang, Xiaozhan., & Pan, Hui (2023). Recent Advances in Electrocatalysts for Efficient Nitrate Reduction to Ammonia. Advanced Functional Materials, 33(43).
MLA Liu, Di,et al."Recent Advances in Electrocatalysts for Efficient Nitrate Reduction to Ammonia".Advanced Functional Materials 33.43(2023).
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